纳微界面增强CO<sub>2</sub>吸收及机理分析

陆小华; 陈义峰; 董依慧; 吉晓燕; 谢文龙; 吴楠桦; 安蓉; 戴中洋; 李峥

doi:10.11949/0438-1157.20191227

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纳微界面增强CO₂吸收及机理分析

综述与专论 | 更新时间：2026-07-24

- 纳微界面增强CO₂吸收及机理分析
- Nano-interface enhanced CO₂ absorption and mechanism analysis
- 化工学报 2020年71卷第1期页码：34-42
- 作者机构：
  
  1. 南京工业大学化工学院，江苏南京 211816
  2. 吕勒奥工业大学能源工程系，瑞典吕勒奥 97187
  3. 南京理工大学材料科学与工程学院，格莱特纳米科学研究所，江苏南京 210094
- 作者简介：
  
  陆小华（1959—），男，博士，教授，xhlu@njtech.edu.cn
- 基金信息：
  
  国家自然科学基金项目(21838004);国家自然科学基金海外及港澳学者合作研究项目(21729601)
- DOI：10.11949/0438-1157.20191227
  中图分类号： TQ 01
- 收稿：2019-10-23，
  
  修回：2019-11-23，
  
  网络首发：2020-08-12，
  
  纸质出版：2020-01-05
- 稿件说明：
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陆小华, 陈义峰, 董依慧, 吉晓燕, 谢文龙, 吴楠桦, 安蓉, 戴中洋, 李峥. 纳微界面增强CO₂吸收及机理分析[J]. 化工学报, 2020, 71(1): 34-42 DOI: 10.11949/0438-1157.20191227.

LU Xiaohua, CHEN Yifeng, DONG Yihui, JI Xiaoyan, XIE Wenlong, WU Nanhua, AN Rong, DAI Zhongyang, LI Zheng. Nano-interface enhanced CO₂ absorption and mechanism analysis[J]. CIESC Journal, 2020, 71(1): 34-42 DOI: 10.11949/0438-1157.20191227.
陆小华, 陈义峰, 董依慧, 吉晓燕, 谢文龙, 吴楠桦, 安蓉, 戴中洋, 李峥. 纳微界面增强CO₂吸收及机理分析[J]. 化工学报, 2020, 71(1): 34-42 DOI: 10.11949/0438-1157.20191227. DOI：

LU Xiaohua, CHEN Yifeng, DONG Yihui, JI Xiaoyan, XIE Wenlong, WU Nanhua, AN Rong, DAI Zhongyang, LI Zheng. Nano-interface enhanced CO₂ absorption and mechanism analysis[J]. CIESC Journal, 2020, 71(1): 34-42 DOI: 10.11949/0438-1157.20191227. DOI：

摘要

捕集与分离是解决当前全球温室效应和发展可再生能源的关键步骤，传统CO

分离及过程强化方法存在速率与效率的博弈。纳微界面强化广泛用于多相传递的化工过程，其对CO

传递过程

的影响也比较显著。本综述从纳微界面处CO

传递模型的建立及阻力调控、纳微界面处CO

平衡态化学位的获取(推动力调控)以及界面强化机制的分子模拟分析等三个方面进行阐述。基于上述结果进一步分析真实吸收塔分离CO

过程的阻力调控并提出“三段式强化方案”，以优化CO

分离过程的投资与运行成本。

Abstract

capture and separation (CCS) is a key step to mitigate greenhouse gas emissions and develop renewable energy. The trade-off between the rate and efficiency in the CO

separation process cannot be solved with the traditional process intensification. Using nano-interface to realize process intensification has been widely used in the chemical process with multi-phase transfer

and CO

separation is one of examples. This review summarizes the research work from the establishment of CO

transfer model at nano-interface and the resistance regulation

the acquisition of the CO

chemical potentials at equilibrium and at the nano-interface (the driving force regulation) and the molecular simulation analysis of the interface enhancement mechanism. Based on the theoretical studies

the resistance distribution for the CO

separation process in a real absorption tower is further analyzed and a “three-stage strengthening scheme” is proposed to decrease the investment and operating costs.

关键词

Keywords

references

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纳微界面增强CO2吸收及机理分析

Nano-interface enhanced CO2 absorption and mechanism analysis

DOI：10.11949/0438-1157.20191227

摘要

Abstract

关键词

Keywords

references

纳微界面增强CO₂吸收及机理分析

Nano-interface enhanced CO₂ absorption and mechanism analysis