天津大学化工学院,化学工程联合国家重点实验室, 天津 300072
刘静(1993—),女,硕士研究生,lj126510@163.com
马友光(1964—),男,博士,教授,ygma@tju.edu.cn
收稿:2019-07-01,
修回:2019-11-05,
网络首发:2020-08-14,
纸质出版:2020-02-05
移动端阅览
刘静, 朱春英, 周灏, 付涛涛, 马友光. 微通道内浆料体系中的气泡生成特性及尺寸预测[J]. 化工学报, 2020, 71(2): 544-551
LIU Jing, ZHU Chunying, ZHOU Hao, FU Taotao, MA Youguang. Bubble formation of slurry system and size prediction in microchannel[J]. CIESC Journal, 2020, 71(2): 544-551
刘静, 朱春英, 周灏, 付涛涛, 马友光. 微通道内浆料体系中的气泡生成特性及尺寸预测[J]. 化工学报, 2020, 71(2): 544-551 DOI: 10.11949/0438-1157.20190745.
LIU Jing, ZHU Chunying, ZHOU Hao, FU Taotao, MA Youguang. Bubble formation of slurry system and size prediction in microchannel[J]. CIESC Journal, 2020, 71(2): 544-551 DOI: 10.11949/0438-1157.20190745.
利用高速摄像仪对T型微通道内浆料体系中的气泡生成频率和气泡尺寸进行了研究。以氮气作为分散相,含0.35%(质量分数)表面活性剂(SDS)不同浓度玻璃珠的甘油-水溶液为连续相。实验考察了弹状流下气液两相流量、颗粒浓度以及浆料表观黏度对气泡生成频率及气泡尺寸的影响。结果表明:在弹状流下,当分散相流量一定时,随着连续相流量的增大,气泡的生成频率增大而气泡尺寸减小。当连续相流量一定时,随着分散相流量的增大,气泡生成频率和气泡尺寸均增大。随着颗粒浓度的增大,浆料的表面张力减小,表观黏度增大,气泡生成频率增大而气泡尺寸减小。提出了T型微通道内浆料体系中生成气泡尺寸的预测模型,模型具有良好的预测精度。
The bubble generation process in liquid-solid slurry system in T-junction microchannel was visually investigated by a high-speed camera. The glycerol-water solutions containing 0.35%(mass) of surfactant (SDS) and different concentrations of glass beads were used as the continuous phase
nitrogen as the dispersed phase. The effects of gas and liquid flow rates
particle concentration and superficial viscosity of slurry on the bubble generation frequency and bubble size under the Taylor flow were studied. The results show that under the Taylor flow regime
when the flow rate of the dispersed phase is constant
the frequency of bubble generation increases but its length decreases with the increase of the flow rate of the continuous phase. As the flow rate of the continuous phase is fixed
both the formation frequency and size of bubble increase with the increase of the flow rate of the dispersed phase. When particle concentration increases
the surface tension decreases of the slurry but its superficial viscosity increases
the bubble generation frequency rises while its size declines. A prediction model for bubble size in the T-type microchannel slurry system is proposed
and the model has good prediction accuracy.
陈光文 , 袁权 . 微化工技术 [J ] . 化工学报 , 2003 , 54 ( 4 ): 427 - 439 .
Chen G W , Yuan Q . Micro chemical technology [J ] . Journal of Chemical Industry and Engineering (China) , 2003 , 54 ( 4 ): 427 - 439 .
骆广生 , 王凯 , 徐建鸿 , 等 . 微化工系统内多相流动及其传递反应性能研究进展 [J ] . 化工学报 , 2010 , 61 ( 7 ): 1621 - 1626 .
Luo G S , Wang K , Xu J H , et al . Multiphase flow, transport and reaction in micro-structured chemical systems [J ] . CIESC Journal , 2010 , 61 ( 7 ): 1621 - 1626 .
荀涛 , 蔡旺锋 , 张旭斌 . 微通道中气-液-液三相流流型及传质研究 [J ] . 化学工业与工程 , 2017 , 34 ( 6 ): 81 - 87 .
Xun T , Cai W F , Zhang X B . The flow pattern and mass transfer of gas-liquid-liquid three phase flow in microchannel [J ] . Chemical Industry and Engineering , 2017 , 34 ( 6 ): 81 - 87 .
Song H , Tice J D , Ismagilov R F . A microfluidic system for controlling reaction networks in time [J ] . Angewandte Chemie International Edition , 2003 , 42 ( 7 ): 768 - 772 .
Laporte M , Montillet A , Della Valle D , et al . Characteristics of foams produced with viscous shear thinning fluids using microchannels at high throughput [J ] . Journal of Food Engineering , 2016 , 173 : 25 - 33 .
Khan S A , Günther A , Schmidt M A , et al . Microfluidic synthesis of colloidal silica [J ] . Langmuir , 2004 , 20 ( 20 ): 8604 - 8611 .
Zhang Y , Ozdemir P . Microfluidic DNA amplification—a review [J ] . Analytica Chimica Acta , 2009 , 638 ( 2 ): 115 - 125 .
Santos J , Trujillo-Cayado L A , Calero N , et al . Development of eco-friendly emulsions produced by microfluidization technique [J ] . Journal of Industrial and Engineering Chemistry , 2016 , 36 : 90 - 95 .
赵绍磊 , 王灵宇 , 吴送姑 . 药物多晶型的研究进展 [J ] . 化学工业与工程 , 2018 , 35 ( 3 ): 12 - 21 .
Zhao S L , Wang L Y , Wu S G . Progress in the research of pharmaceutical polymorph [J ] . Chemical Industry and Engineering , 2018 , 35 ( 3 ): 12 - 21
Qian D , Lawal A . Numerical study on gas and liquid slugs for Taylor flow in a T-junction microchannel [J ] . Chemical Engineering Science , 2006 , 61 ( 23 ): 7609 - 7625 .
Sobieszuk P , Cygański P , Pohorecki R . Bubble lengths in the gas-liquid Taylor flow in microchannels [J ] . Chemical Engineering Research and Design , 2010 , 88 ( 3 ): 263 - 269 .
Garstecki P , Fuerstman M J , Stone H A , et al . Formation of droplets and bubbles in a microfluidic T-junction—scaling and mechanism of break-up [J ] . Lab on a Chip , 2006 , 6 ( 3 ): 437 - 446 .
Ookawara S , Street D , Ogawa K . Numerical study on development of particle concentration profiles in a curved microchannel [J ] . Chemical Engineering Science , 2006 , 61 ( 11 ): 3714 - 3724 .
Ai Y , Park S , Zhu J , et al . DC electrokinetic particle transport in an L-shaped microchannel [J ] . Langmuir , 2010 , 26 ( 4 ): 2937 - 2944 .
Khashan S A , Furlani E P . Effects of particle-fluid coupling on particle transport and capture in a magnetophoretic microsystem [J ] . Microfluidics and Nanofluidics , 2012 , 12 ( 1 ): 565 - 580 .
Luo G , Du L , Wang Y , et al . Controllable preparation of particles with microfluidics [J ] . Particuology , 2011 , 9 ( 6 ): 545 - 558 .
Wang K , Wang Y J , Chen G G , et al . Enhancement of mixing and mass transfer performance with a microstructure minireactor for controllable preparation of CaCO 3 nanoparticles [J ] . Industrial & Engineering Chemistry Research , 2007 , 46 ( 19 ): 6092 - 6098 .
Ufer A , Sudhoff D , Mescher A , et al . Suspension catalysis in a liquid-liquid capillary microreactor [J ] . Chemical Engineering Journal , 2011 , 167 ( 2 ): 468 - 474 .
谢灵丹 . 微通道内微细颗粒对气液传质的影响研究 [D ] . 天津 : 天津大学 , 2010 .
Xie L D . Effect of fine particle on the gas-liquid mass transfer in the microchannel [D ] . Tianjin : Tianjin University , 2010 .
Pu X , Su Y . Heterogeneous catalysis in microreactors with nanofluids for fine chemicals syntheses: benzylation of toluene with benzyl chloride over silica-immobilized FeCl 3 catalyst [J ] . Chemical Engineering Science , 2018 , 184 : 200 - 208 .
Pu X , Zhang B , Su Y . Heterogeneous photocatalysis in microreactors for efficient reduction of nitrobenzene to aniline: mechanisms and energy efficiency [J ] . Chemical Engineering & Technology , 2019 , 42 ( 10 ): 1 - 9 .
Chen R , Feng H , Zhu X , et al . Interaction of the Taylor flow behaviors and catalytic reaction inside a gas-liquid-solid microreactor under long-term operation [J ] . Chemical Engineering Science , 2018 , 175 : 175 - 184 .
Bashir S , Solvas X C , Bashir M , et al . Dynamic wetting in microfluidic droplet formation [J ] . BioChip Journal , 2014 , 8 ( 2 ): 122 - 128 .
Riaud A , Zhang H , Wang X , et al . Numerical study of surfactant dynamics during emulsification in a T-junction microchannel [J ] . Langmuir , 2018 , 34 ( 17 ): 4980 - 4990 .
Tsuchiya K , Furumoto A , Fan L S , et al . Suspension viscosity and bubble rise velocity in liquid-solid fluidized beds [J ] . Chemical Engineering Science , 1997 , 52 ( 18 ): 3053 - 3066 .
Yang G Q , Du B , Fan L S . Bubble formation and dynamics in gas-liquid-solid fluidization—a review [J ] . Chemical Engineering Science , 2007 , 62 ( 1/2 ): 2 - 27 .
Dayan A , Zalmanovich S . Axial dispersion and enterainment of particles in wakes of bubbles [J ] . Chemical Engineering Science , 1982 , 37 ( 8 ): 1253 - 1257 .
Garstecki P , Stone H A , Whitesides G M . Mechanism for flow-rate controlled breakup in confined geometries: a route to monodisperse emulsions [J ] . Physical Review Letters , 2005 , 94 ( 16 ): 164501 .
Fu T , Ma Y , Funfschilling D , et al . Bubble formation and breakup mechanism in a microfluidic flow-focusing device [J ] . Chemical Engineering Science , 2009 , 64 ( 10 ): 2392 - 2400 .
Christopher G F , Noharuddin N N , Taylor J A , et al . Experimental observations of the squeezing-to-dripping transition in T-shaped microfluidic junctions [J ] . Physical Review E , 2008 , 78 ( 3 ): 036317 .
Xu J H , Li S W , Tan J , et al . Correlations of droplet formation in T-junction microfluidic devices: from squeezing to dripping [J ] . Microfluidics and Nanofluidics , 2008 , 5 ( 6 ): 711 - 717 .
Fu T , Ma Y , Funfschilling D , et al . Squeezing-to-dripping transition for bubble formation in a microfluidic T-junction [J ] . Chemical Engineering Science , 2010 , 65 ( 12 ): 3739 - 3748 .
Nisisako T , Torii T , Higuchi T . Droplet formation in a microchannel network [J ] . Lab on a Chip , 2002 , 2 ( 1 ): 24 - 26 .
Xu J H , Luo G S , Chen G G , et al . Experimental and theoretical approaches on droplet formation from a micrometer screen hole [J ] . Journal of Membrane Science , 2005 , 266 ( 1/2 ): 121 - 131 .
0
浏览量
0
下载量
1
CSCD
关联资源
相关文章
相关作者
相关机构
京公网安备11010102001995号