YUAN Xuemei, DENG Shihuai, YANG Yuesuo, et al. Effects of granular size and flow rate on transport of silver nanoparticles in saturated porous media[J]. CIESC Journal, 2017, (11): 4154-4160.
DOI:
YUAN Xuemei, DENG Shihuai, YANG Yuesuo, et al. Effects of granular size and flow rate on transport of silver nanoparticles in saturated porous media[J]. CIESC Journal, 2017, (11): 4154-4160.DOI: 10.11949/j.issn.0438-1157.20170282.
Effects of granular size and flow rate on transport of silver nanoparticles in saturated porous media
Being one of the most widely used engineered nanomaterials well known for its ecological toxicity
silver nanoparticles have big potential to arise severe environmental problems on entry groundwater environment. Unfortunately
thus far how environmental factors may control the mobility of silver nanparticles remain unclear. In this study
column experiments were employed to investigate the interplay of flow rate (1 and 2 ml·min-1) and granular size characteristics (glass beads of 0.605
0.115 mm
and the mixture of the two) on the transport of nano silver in saturated porous media. The results suggested that transport of silver nanoparticles in the matrix of large grains (0.605 mm) was controlled mainly by deposition while that in the other two matrix (0.115 mm and the mixture) was controlled by both the deposition and straining processes. For the matrix of the mixed grains
straining was mainly controlled by the fraction of the grains with lower size. Increasing flow rate reduced deposition of the nanoparticles in the matrix with large grains
while for the other two matrices (with small grains or mixed grains)
increasing flow rate reduced not only the deposition rate but also the straining rate
resulting in a more significant reduction in particle attenuation by the porous medium. Moreover
the intensified size exclusion effect accompanied by the rising flow rate can also increase the transport velocity of the silver nanoparticles in the matrix of small and mixed grains. These findings were critical to understanding the movement and distribution of nanomaterials in dynamic and complex groundwater environment.
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Related Author
LING Chen
JIANG Xin
WANG Zhiyong
QIN Xiangfei
LU Jiangang
YE Xueyan
DU Xinqiang
ZHANG Hexuan
Related Institution
Zhejiang Provincial Key Laboratory of Advanced Chemical Engineering Manufacture Technology, College of Chemical and Biological Engineering, Zhejiang University
State Key Laboratory of Industrial Control Technology, Department of Control Science and Engineering, Zhejiang University
Key Laboratory of Groundwater Resources and Environment, Ministry of Education, Jilin University
College of Resources and Environment, Jilin University