Nano-interface enhanced CO<sub>2</sub> absorption and mechanism analysis

LU Xiaohua; CHEN Yifeng; DONG Yihui; JI Xiaoyan; XIE Wenlong; WU Nanhua; AN Rong; DAI Zhongyang; LI Zheng

doi:10.11949/0438-1157.20191227

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Nano-interface enhanced CO₂ absorption and mechanism analysis

Reviews and monographs | 更新时间：2026-07-24

- Nano-interface enhanced CO₂ absorption and mechanism analysis
- CIESC Journal Vol. 71, Issue 1, Pages: 34-42(2020)
- 作者机构：
  
  1. 南京工业大学化工学院，江苏南京 211816
  2. 吕勒奥工业大学能源工程系，瑞典吕勒奥 97187
  3. 南京理工大学材料科学与工程学院，格莱特纳米科学研究所，江苏南京 210094
- 作者简介：
- 基金信息：
- DOI：10.11949/0438-1157.20191227
  CLC： TQ 01
- Received：23 October 2019，
  
  Revised：2019-11-23，
  
  Online First：12 August 2020，
  
  Published：05 January 2020
- 稿件说明：
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陆小华, 陈义峰, 董依慧, 吉晓燕, 谢文龙, 吴楠桦, 安蓉, 戴中洋, 李峥. 纳微界面增强CO₂吸收及机理分析[J]. 化工学报, 2020, 71(1): 34-42 DOI: 10.11949/0438-1157.20191227.

LU Xiaohua, CHEN Yifeng, DONG Yihui, JI Xiaoyan, XIE Wenlong, WU Nanhua, AN Rong, DAI Zhongyang, LI Zheng. Nano-interface enhanced CO₂ absorption and mechanism analysis[J]. CIESC Journal, 2020, 71(1): 34-42 DOI: 10.11949/0438-1157.20191227.
陆小华, 陈义峰, 董依慧, 吉晓燕, 谢文龙, 吴楠桦, 安蓉, 戴中洋, 李峥. 纳微界面增强CO₂吸收及机理分析[J]. 化工学报, 2020, 71(1): 34-42 DOI: 10.11949/0438-1157.20191227. DOI：

LU Xiaohua, CHEN Yifeng, DONG Yihui, JI Xiaoyan, XIE Wenlong, WU Nanhua, AN Rong, DAI Zhongyang, LI Zheng. Nano-interface enhanced CO₂ absorption and mechanism analysis[J]. CIESC Journal, 2020, 71(1): 34-42 DOI: 10.11949/0438-1157.20191227. DOI：

摘要

捕集与分离是解决当前全球温室效应和发展可再生能源的关键步骤，传统CO

分离及过程强化方法存在速率与效率的博弈。纳微界面强化广泛用于多相传递的化工过程，其对CO

传递过程

的影响也比较显著。本综述从纳微界面处CO

传递模型的建立及阻力调控、纳微界面处CO

平衡态化学位的获取(推动力调控)以及界面强化机制的分子模拟分析等三个方面进行阐述。基于上述结果进一步分析真实吸收塔分离CO

过程的阻力调控并提出“三段式强化方案”，以优化CO

分离过程的投资与运行成本。

Abstract

capture and separation (CCS) is a key step to mitigate greenhouse gas emissions and develop renewable energy. The trade-off between the rate and efficiency in the CO

separation process cannot be solved with the traditional process intensification. Using nano-interface to realize process intensification has been widely used in the chemical process with multi-phase transfer

and CO

separation is one of examples. This review summarizes the research work from the establishment of CO

transfer model at nano-interface and the resistance regulation

the acquisition of the CO

chemical potentials at equilibrium and at the nano-interface (the driving force regulation) and the molecular simulation analysis of the interface enhancement mechanism. Based on the theoretical studies

the resistance distribution for the CO

separation process in a real absorption tower is further analyzed and a “three-stage strengthening scheme” is proposed to decrease the investment and operating costs.

关键词

Keywords

references

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⁰

Nano-interface enhanced CO2 absorption and mechanism analysis

DOI：10.11949/0438-1157.20191227

摘要

Abstract

关键词

Keywords

references

Nano-interface enhanced CO₂ absorption and mechanism analysis