KINETIC STUDIES ON THE OXIDATION OF SULFUR DIOXIDE ON VANADIUM CATALYST ——Ⅲ.  A COMPARISON OF THE RATE EQUATIONS OBTAINED WITH SOME INDUSTRIAL VANADIUM CATALYSIS

CHANG MAN-CHEN; Kuo SHEN-TU AND WANG SHIH-CHUN (Institute of Applied Chemistry; Academia Sinica)

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KINETIC STUDIES ON THE OXIDATION OF SULFUR DIOXIDE ON VANADIUM CATALYST ——Ⅲ. A COMPARISON OF THE RATE EQUATIONS OBTAINED WITH SOME INDUSTRIAL VANADIUM CATALYSIS

更新时间：2025-12-16

- KINETIC STUDIES ON THE OXIDATION OF SULFUR DIOXIDE ON VANADIUM CATALYST ——Ⅲ. A COMPARISON OF THE RATE EQUATIONS OBTAINED WITH SOME INDUSTRIAL VANADIUM CATALYSIS
- CIESC Journal Issue 2, (1959)
- 作者机构：
  
  中国科学院应用化学研究所,中国科学院应用化学研究所,中国科学院应用化学研究所
- 作者简介：
- 基金信息：
- DOI：
  CLC：
- Online First：25 December 1959，
  
  Published：25 December 1959
- 稿件说明：
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CHANG MAN-CHEN, Kuo SHEN-TU AND WANG SHIH-CHUN (Institute of Applied Chemistry, Academia Sinica). KINETIC STUDIES ON THE OXIDATION OF SULFUR DIOXIDE ON VANADIUM CATALYST ——Ⅲ. A COMPARISON OF THE RATE EQUATIONS OBTAINED WITH SOME INDUSTRIAL VANADIUM CATALYSIS[J]. CIESC Journal, 1959, (2).
DOI：

CHANG MAN-CHEN, Kuo SHEN-TU AND WANG SHIH-CHUN (Institute of Applied Chemistry, Academia Sinica). KINETIC STUDIES ON THE OXIDATION OF SULFUR DIOXIDE ON VANADIUM CATALYST ——Ⅲ. A COMPARISON OF THE RATE EQUATIONS OBTAINED WITH SOME INDUSTRIAL VANADIUM CATALYSIS[J]. CIESC Journal, 1959, (2). DOI：

摘要

作者等过去的工作已经证实

由于扩散过程的影响、温度范围的不同、或化学组成的差异

二氧化硫在钒催化剂上的氧化动力学方程式可能具有不同的形式。反应物及生成物与催化剂之间的相互作用

可能使催化剂具有不同的颜色与活性

因而即使温度相同

由于催化剂在层内所处的部位不同

其催化活性可能并不一致。这些复杂性给工业设计带来了很大的困难。因此

合理的简化是完全必要的。作者等选取了几种不同的工业钒催化剂

用实验方法求得了适用于它们的动力学方程式

进行比较和讨论

提出了一个简便的、合理的、可以用作设计基础的动力学方程式。

Abstract

Rate equations obtained with a number of industrial vanadium catalysts for the oxidation of sulfur dioxide showed the complicacy of the kinetics of the reaction. .Although the theoretical rate equation for this catalytic process remains uncertain

among emperical equations the following is prefer for design purposes:

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