Cycled storage-discharge plasma catalytic process for toluene removal from indoor air
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Cycled storage-discharge plasma catalytic process for toluene removal from indoor air
CIESC JournalIssue 7, (2011)
作者机构:
大连理工大学等离子体物理化学实验室
作者简介:
基金信息:
DOI:
CLC:
Online First:05 July 2011,
Published:05 July 2011
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范红玉. Cycled storage-discharge plasma catalytic process for toluene removal from indoor air[J]. CIESC Journal, 2011, (7).
DOI:
范红玉. Cycled storage-discharge plasma catalytic process for toluene removal from indoor air[J]. CIESC Journal, 2011, (7).DOI:
Cycled storage-discharge plasma catalytic process for toluene removal from indoor air
摘要
Abstract
Non-thermal plasmas(NTPs)technique has a great potential for indoor air purification
however
the high energy cost and secondary pollutants formation limit its practical application. To resolve these problems
a cycled storage-discharge(CSD)plasma catalytic process was explored for the removal of low-concentration toluene from indoor air in this study. The performance of toluene storage and plasma catalytic oxidation of adsorbed-state toluene over non-loaded and silver-loaded HZSM-5 catalysts was investigated. The experimental results showed that silver-loaded HZSM-5 catalysts gave a longer breakthrough time than non-loaded HZSM-5 catalysts at the storage stage(storage condition: 0.1 g·m-3 C7H8
40% relative humidity(RH
25℃)
2000 ml·min-1 flow rate of simulated air).With input power of 40 W
the adsorbed-state toluene could be almost oxidized to CO2 in 10 min at the discharge stage(carbon balance about 100%
CO2 selectivity 98.2%).It was further proved that there was no toluene desorbed during the process of plasma catalytic oxidation by on-line detection with mass spectrometry(MS)and Fourier transform infrared spectrometry(FTIR).Preliminary investigation on the stability of the CSD process for toluene removal was conducted. This study provides a novel plasma catalytic process for removing toluene from indoor air.