CIESC Journal ›› 2018, Vol. 69 ›› Issue (7): 3059-3067.doi: 10.11949/j.issn.0438-1157.20171620

Previous Articles     Next Articles

Characteristics of p-nitrophenol removal by SAT system with iron oxide coated sands

WEN Yujuan1, YANG Yuesuo1,2, SONG Xiaoming1, ZHANG Xi2, LI Huizhong3   

  1. 1 Key Laboratory of Regional Environment and Eco-restoration, Ministry of Education, Shenyang University, Shenyang 110044, Liaoning, China;
    2 Key Laboratory of Groundwater Resources and Environment, Ministry of Education, Jilin University, Changchun 130021, Jilin, China;
    3 Geological and Environmental Monitoring Station of Liaoning Province, Shenyang 110032, Liaoning, China
  • Received:2017-12-08 Revised:2018-01-18 Online:2018-07-05 Published:2018-01-29
  • Supported by:

    supported by the National Natural Science Foundation of China (41703125, 41472237) and Liaoning Province Innovation Team Project(LT201502).

PDF (PC)

84

Abstract:

The more and more nitro aromatic compounds have been detected in the environment, and one of the most popular compounds was p-nitrophenol. To improve the removal effect of p-nitrophenol using soil aquifer system (SAT), the system was innovated with iron-oxide coated sand as the aquifer media. Characterization of the iron coated SAT shows that surface of the oxidized iron film was flocculent or lamellar without fixed shape. Ironoxide coated sand has pore structure and makes the specific surface increased 2 times to 4 times. Study of absorption kinetics indicated that the absorption kinetics were governed by the Freundlich model of chemical adsorption, and the absorption capacity was much enhanced. The diffusion model study demonstrated the pore diffusion was higher than sufficient diffusion. The results of the mini-column break through show that the adsorption is closely related to the residence time of the solute in the medium, so the flow rate should be appropriately controlled during the SAT operation.

Key words: SAT, pollution, regeneration, kinetics, diffusion model

CLC Number: 

  • X523

[1] NAUMANN J C, ANDERSON J E, YOUNG D R. Remote detection of plant physiological responses to TNT soil contamination[J]. Plant and Soil, 2010, 329(1/2):239-248.
[2] ZOHAR S, KVIATKOVSKI I, MASAPHY S. Increasing tolerance to and degradation of high p-nitrophenol concentrations by inoculum size manipulations of Arthrobacter 4Hβ isolated from agricultural soil[J]. International Biodeterioration & Biodegradation, 2013, 84:80-85.
[3] CHEN J, SONG M, LI Y, et al. The effect of phytosterol protects rats against 4-nitrophenol-induced liver damage[J]. Environmental Toxicology and Pharmacology, 2016, 41:266-271.
[4] MEGHARAJ M, PEARSON H W, VENKATESWARLU K. Toxicity of phenol and three nitrophenols towards growth and metabolic activities of Nostoc linckia, isolated from soil[J]. Archives of Environmental Contamination and Toxicology, 1991, 21(4):578-584.
[5] KUDA T, KYOI D, TAKAHASHI H, et al. Detection and isolation of p-nitrophenol-lowering bacteria from intestine of marine fishes caught in Japanese waters[J]. Marine Pollution Bulletin, 2011, 62(8):1622-1627.
[6] NAKATSUJI Y, SALEHI Z, KAWASE Y. Mechanisms for removal of p-nitrophenol from aqueous solution using zero-valent iron[J]. Journal of Environmental Management, 2015, 152:183-191.
[7] KIM T S, KIM J K, CHOI K, et al. Degradation mechanism and the toxicity assessment in TiO2 photocatalysis and photolysis of parathion[J]. Chemosphere, 2006, 62(6):926-933.
[8] 傅厚暾, 赵俐敏, 冯娟, 等. Fenton试剂-超声波降解对硝基苯胺产物的分析[J]. 江汉大学学报(自然科学版), 2004, (2):74-76. FU H D, ZHAO L M, FENG J, et al. Determination of Fentonultrasonic degradation products of p-nitroaniline[J]. Journal of Jianghan University(Natural Science Edition), 2004, (2):74-76.
[9] 宋瀚文, 王东红, 徐雄, 等. 我国24个典型饮用水源地中14种酚类化合物浓度分布特征[J]. 环境科学学报, 2014, 34(2):355-362. SONG H W, WANG D H, XU X, et al. Occurrence of 14 phenols in 24 typical drinking water sources of China[J]. Acta Scientiae Circumstantiae, 2014, 34(2):355-362.
[10] 辛苗苗, 危起伟, 王志坚, 等. 对硝基酚对稀有鲫胚胎的急性毒性[J]. 淡水渔业, 2014, (5):43-48. XIN M M, WEI Q W, WANG Z J, et al. Acute toxicity of p-nitrophenol to Gobiocypris raruse[J]. Freshwater Fisheries, 2014, (5):43-48.
[11] DUSTER T A, NA C, BOLSTER D, et al. Transport of single-layered graphene oxide nanosheets through quartz and iron oxide-coated sand columns[J]. Journal of Environmental Engineering, 2016, 4(1):60-79
[12] YANG X, FLYNN R, VON DER KAMMER F, et al. Influence of ionic strength and pH on the limitation of latex microsphere deposition sites on iron-oxide coated sand by humic acid[J]. Environmental Pollution, 2011, 159(7):1896-1904.
[13] ALVAREZ-SILVA M, MIRNEZAMI M, URIBE-SALAS A, et al. Point of zero charge, isoelectric point and aggregation of phyllosilicate minerals[J]. Canadian Metallurgical Quarterly, 2010, 49(4):405-410
[14] KILISLIOGLU A, BILGIN B. Thermodynamic and kinetic investigations of uranium adsorption on amberlite IR-118H resin[J]. Applied Radiation and Isotopes, 2003, 58(2):155-160.
[15] KRAUSS M, WILCKE W, KOBZA J, et al. Predicting heavy metal transfer from soil to plant:potential use of Freundlich -type functions[J]. Journal of Plan Nutrition and Soil Science, 2002, 165(1):3-8.
[16] JAIN M, GARG V K, KADIRVELU K, et al. Adsorption of heavy metals from multi-metal aqueous solution by sunflower plant biomassbased carbons[J]. International Journal of Environmental Science and Technology, 2016, 13(2):493-500.
[17] MIYITTAH M K, TSYAWO F W, KUMAH K K, et al. Suitability of two methods for determination of point of zero charge (PZC) of adsorbents in soils[J]. Communications in Soil Science and Plant Analysis, 2016, 47(1):101-111.
[18] 佟迪, 于海华. 不同滤料载体改性机理研究[J]. 辽宁化工, 2010, (5):514-516. TONG D, YU H H. Study on the modification mechanism of different filter carriers[J]. Liaoning Chemical Industry, 2010, (5):514-516.
[19] 张建锋, 魏宁, 王晓昌. 改性滤料氟吸附性能对比研究[J]. 西安建筑科技大学学报(自然科学版), 2007, 39(6):850-855. ZHANG J F, WEI N, WANG X C. Adsorption of fluoride from water by preparing coated media[J]. Journal of Xi'an University of Architecture & Technology (Natural Science Edition), 2007, 39(6):850-855.
[20] NIU M, WU M, LV Y, et al. Powder activated carbon to the West Lake Gui sudden fluoroquinolone antibiotics (NOR) pollution removal research[J]. International Journal of Ecology, 2016, 5(3):34-48.
[21] 方圣琼, 潘进, 李晓, 等. 羟基铁柱撑蒙脱石对庆大霉素的吸附性能[J]. 硅酸盐学报, 2016, 44(2):314-321. FANG S Q, PAN J, LI X, et al. Adsorption property of gentamicin on hydroxy-Fe intercalated montmorillonite[J]. Journal of the Chinese Ceramic Society, 2016, 44(2):314-321.
[22] 郝全龙, 谯华, 周从直, 等. 富里酸对TNT的吸附-解吸行为[J]. 环境工程学报, 2016, 10(5):2687-2692. HAO Q L, QIAO H, ZHOU C Z, et al. Adsorption and desorption behaviors of TNT on fulvic acid[J]. Chinese Journal of Environmental Engineering, 2016, 10(5):2687-2692.
[23] KUMAR P S, SARAVANAN A, KUMAR K A, et al. Removal of toxic zinc from water/wastewater using eucalyptus seeds activated carbon:non-linear regression analysis[J]. IET Nanobiotechnology, 2016, 10(4):244.
[24] DAHDAL Y N, OREN Y, SCHWAHN D, et al. Biopolymer-induced calcium phosphate scaling in membrane-based water treatment systems:Langmuir model films studies[J]. Colloids and Surfaces B:Biointerfaces, 2016, 143:233-242.
[25] OZKAYA B. Adsorption and desorption of phenol on activated carbon and a comparison of isotherm models[J]. Journal of Hazardous Materials, 2006, 129(1):158-163.
[26] LAI C H, CHEN C Y. Removal of metal ions and humic acid from water by iron-coated filter media[J]. Chemosphere, 2001, 44(5):1177-1184.
[27] JAIN M, GARG V K, KADIRVELU K, et al. Adsorption of heavy metals from multi-metal aqueous solution by sunflower plant biomassbased carbons[J]. International Journal of Environmental Science and Technology, 2016, 13(2):493-500.
[28] CHAUHAN A, CHAKRABORTI A K, JAIN R K. Plasmid-encoded degradation of p-nitrophenol and 4-nitrocatechol by Arthrobacter protophormiae[J]. Biochemical and Biophysical Research Communications, 2000, 270(3):733-740.
[1] LI Desheng, ZHANG Chao, DENG Shihai, HU Zhifeng, LI Jinlong, LIU Yuanhui. Experimental study on effective nitrate removal from sewage by ZVI-based catalyzed reduction [J]. CIESC Journal, 2019, 70(3): 1065-1074.
[2] ZHOU Xuebing, LIU Chanjuan, LUO Jinqiong, LIANG Deqing. Microscopic measurements on methane hydrate dissociation [J]. CIESC Journal, 2019, 70(3): 1042-1047.
[3] LI Yanying, LI Xianchun. Biomass activated carbon loaded with zero-valent iron nanocrystal clusters for direct catalytic reduction of NO [J]. CIESC Journal, 2019, 70(3): 1111-1119.
[4] ZHANG Hang, WENG Jianhua, CUI Xiaoyu. Heat transfer performance of pulsating heat pipe with hygroscopic salt solution [J]. CIESC Journal, 2019, 70(3): 874-882.
[5] HUANG Weiqing, XU Pingru, QIAN Yu. Atmospheric environment risk analysis of oil consuming by vehicles based on FTA method: taking Hangzhou as a case study [J]. CIESC Journal, 2019, 70(2): 661-669.
[6] XUE Yongfei, WANG Yalin, SUN Bei, LI Qianzhong, SUN Jiazhou. Improved state transfer algorithm-based kinetics parameter estimation for cascaded plug flow reactors [J]. CIESC Journal, 2019, 70(2): 607-616.
[7] SU Hui, ZHU Zhaowu, WANG Lina, QI Tao. Research progress in extraction and recovery of lithium from hard-rock ores [J]. CIESC Journal, 2019, 70(1): 10-23.
[8] WEN Xiantai, YU Jiao, CAO Xianqi, YU Pengfei, CAI Ning, MAO Yifan. Experimental study of a novel solution regeneration system for heat-source tower under unsteady state [J]. CIESC Journal, 2019, 70(1): 83-90.
[9] XUE Chao, MAO Yanpeng, WANG Wenlong, SONG Zhanlong, ZHAO Xiqiang, SUN Jing, WANG Yanxiang. Treatment of phenol wastewater by microwave catalytic wet oxidation under high pressure [J]. CIESC Journal, 2018, 69(S2): 210-217.
[10] WANG Mu, YIN Yonggao, GUO Xiaoshuang, CHEN Tingting. Alternative scheme and dehumidification and regeneration performance validation for economic multi-component solution [J]. CIESC Journal, 2018, 69(S2): 420-424.
[11] ZOU Huiming, LI Xuan, TANG Mingsheng, SHAO Shuangquan, TIAN Changqing. Experimental investigation on refrigeration performance of R290 linear compressor [J]. CIESC Journal, 2018, 69(S2): 480-484.
[12] XU Jiaxing, CHAO Jingwei, LI Tingxian, WANG Ruzhu. Preparation and characterization of expanded graphite/metal organic frameworks composite sorbent [J]. CIESC Journal, 2018, 69(S2): 492-499.
[13] CHEN Liang, ZHAO Fan, YAN Guangjing, WANG Chunbo. Synergetic effect of H2O and SO2 on calcination kinetics of limestone during simultaneous calcination/sulfation reaction in CFB boilers [J]. CIESC Journal, 2018, 69(9): 3859-3868.
[14] YAN Yan, DONG Jixian. Condensation heat transfer characteristic and flow pattern of steam in rectangular tube with different aspect ratio [J]. CIESC Journal, 2018, 69(9): 3851-3858.
[15] ZHONG Yingjie, HUANG Qi, DENG Kai, ZHAO Chuangyao, SU Yihua. Analysis of flow characteristics in triangular grooved channel by pulsating flow at low Reynolds number [J]. CIESC Journal, 2018, 69(9): 3806-3813.
Viewed
Full text


Abstract

Cited
  Shared   
  Discussed   
No Suggested Reading articles found!
Copyright © 2019 CIESC Journal, All Rights Reserved.
Powered by Beijing Magtech Co. Ltd